纺织学报 ›› 2022, Vol. 43 ›› Issue (05): 185-194.doi: 10.13475/j.fzxb.20210301910

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纺织基柔性染料敏化太阳能电池的研究进展

韩宜君1, 许君1(), 畅琪琪1, 张诚2,3   

  1. 1.天津工业大学 纺织科学与工程学院, 天津 300387
    2.天津工业大学 电子与信息工程学院, 天津 300387
    3.天津市光电检测技术与系统重点实验室, 天津 300387
  • 收稿日期:2021-03-04 修回日期:2021-09-08 出版日期:2022-05-15 发布日期:2022-05-30
  • 通讯作者: 许君
  • 作者简介:韩宜君(1996—),男,硕士生。主要研究方向为纺织基柔性染料敏化太阳能电池。
  • 基金资助:
    天津市“项目+团队”重点培养专项项目(XB202007);天津市重点研发计划科技支撑重点项目(19YFZCSY00180);天津市科技军民融合重大专项项目(18ZXJMTG00260)

Research progress in textile-based flexible dye-sensitized solar cells

HAN Yijun1, XU Jun1(), CHANG Qiqi1, ZHANG Cheng2,3   

  1. 1. School of Textile Science and Engineering, Tiangong University, Tianjin 300387, China
    2. School of Electronic and Information Engineering, Tiangong University, Tianjin 300387, China
    3. Tianjin Key Laboratory of Optoelectronic Detection Technology and System, Tianjin 300387, China
  • Received:2021-03-04 Revised:2021-09-08 Published:2022-05-15 Online:2022-05-30
  • Contact: XU Jun

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摘要：

柔性染料敏化太阳能电池可为可穿戴设备解决供电问题并实现服装一体化,同时能减少能源消耗。为全面探究纺织基柔性染料敏化太阳能电池在纺织领域的应用前景,首先简述了染料敏化太阳能电池的发展现状、主要组成结构、工作机制和性能评价方法,重点介绍了柔性纤维状电池与纺织基底平面电池的研究进展;其次,通过分析电极制备与电池组装方式的特点,指出在当前纺织领域尚未解决的太阳能电池问题,同时总结了纺织基柔性染料敏化太阳能电池电解质与敏化染料的研究进展;最后指出电池电极、染料以及电解质的发展方向,并对纺织基柔性染料敏化太阳能电池的发展提出展望。

关键词: 染料敏化太阳能电池, 纺织基, 电极材料, 织物涂覆, 纤维

Abstract:

Solar energy is one of the effective solutions for the energy problem. Flexible solar cells can solve the power supply problem for wearable devices, and at the same time can facilitate the integration with clothing. In order to comprehensively explore the application prospects of textile-based flexible dye-sensitized solar cells, the development status, composition structure, working mechanism and performance evaluation of dye-sensitized solar cells were reviewed, focusing on the research results of flexible fibrous batteries and textile-based planar batteries, and on analysis of the characteristics of electrode preparation and battery assembly methods. The review also pointed out the unresolved problems in the textile field, and also summarized the development process in textile-based flexible dye-sensitized solar cell electrolytes and sensitizing dyes. It is concluded that the prospect of the development of textile-based flexible dye-sensitized solar cells was put forward.

Key words: dye-sensitized solar cells, textile-based, electrode material, fabric coating, fiber

中图分类号: 

  • TM914.4

图1

正面、背面透光型DSSCs结构示意图 注:HOMO指最高占据分子轨道; LUMO指最低未占分子轨道。"

图2

纤维状DSSCs结构示意图"

图3

“TiO2~I-/ I 3 -~Pt”型DSSCs以及DSSCs工作原理、电子转移过程示意图 注:FTO为导电玻璃;ECB为导带的电势;LUMO为最低未占分子轨道;HOMO为最高占据分子轨道。"

表1

柔性纤维状染料敏化太阳能电池的光伏参数"

电池形态 电池材料组成 电极材料
制备方法		 短路电流/
(mA·cm-2)		 开路电
压/V		 影响因
子F		 光电转化
效率/%		 参考
文献
线状 钛丝/TiO2/N719/I-- I 3 -/铂丝 涂覆法 11.06 0.734 0.672 5.41 [13]
碳纳米管丝/TiO2/N719/I-- I 3 -/碳纳米管丝 化学浴沉积法 — — — 7.6 [15]
碳纳米管丝/N719/I-- I 3 -/碳纳米管/聚偏氟乙烯丝 化学气相沉积法 9.84 0.69 0.57 3.90 [18]
碳纳米管丝/TiO2/N719/I-- I 3 -/碳纳米管丝 涂覆法 — — — 2.94 [19]
网状 钛丝/TiO2/N719/I-- I 3 -/多壁碳纳米管丝 化学气相沉积法 16.0 0.71 0.61 7.13 [20]
缎纹网状 不锈钢丝/ZnO/N719/固体电解质/Pt/不锈钢丝 水热合成法 20.2 0.45 0.28 2.57 [17]

表2

柔性织物基底染料敏化太阳能电池的光伏参数"

电池形态 电池材料组成 电极材料
制备方法		 短路电流/
(mA·cm-2)		 开路电
压/V		 影响因
子FF		 光电转化
效率/%		 参考
文献
全柔平面 玻璃纤维织物/PA层/Ti/TiO2/染料/电解质/聚萘二甲酸乙二醇酯/Pt/ITO 丝网印刷高温烧结 5.7 0.71 0.541 1.8 [24]
机织涤纶/棉(65/35)面料/导电银浆/Ruthenizer 535-bisTBA染料敏化剂/I-- I 3 -/石墨/ITO 丝网印刷低温工艺 9.6 0.67 0.50 3.24 [27]
玻璃纤维织物/导电银浆/TiO2/Ruthenizer 535-bisTBA染料敏化剂/I-- I 3 -/石墨/ITO 丝网印刷低温工艺 10.24 0.73 0.54 4.04 [27]
镀锡铜丝制成的金属微丝纺织品/TiO2/N3/I-- I 3 -/Pt/聚乙烯薄膜 涂覆法高温烧结 0.84 0.41 0.57 0.20 [28]
不锈钢(SUS304)金属织物/TiO2/N719/I-- I 3 -/Pt/活性碳粉/不锈钢金属网 丝网印刷热处理 — — — 2.63 [29]
不锈钢(SUS304)金属织物/TiO2/N719/I-- I 3 -/Pt/活性碳粉/不锈钢金属网 浮动印刷热处理 6.32 0.792 0.67 4.16 [30]
304不锈钢网/TiO2/N719/ I-- I 3 -/Pt/不锈钢网/丝绸 电镀沉积 19.70 0.69 0.43 5.8 [31]
半柔平面 标准涤纶/棉(65/35)织物/导电银浆/TiO2/N719/I-- I 3 -/Pt/FTO 丝网印刷低温工艺 36.56 0.3 0.25 2.78 [26]
纸质基材/Ni/ZnO/N719/I-- I 3 -/Pt/FTO 刮涂法 6.70 0.56 0.33 1.21 [33]
FTO/TiO2/N719/I-- I 3 -/氧化石墨烯/棉织物 涂覆法 9.08 0.64 0.429 7 2.52 [32]
FTO/TiO2/D719/I-- I 3 -/多壁碳纳米管涂层/涤纶织物 流延法空气干燥 11.92 0.688 0.693 9 5.69 [33]
FTO/TiO2/N719/I-- I 3 -/活性炭掺杂多壁碳纳米管/涤纶机织物 刮涂法空气干燥 12.03 0.766 0.790 3 7.29 [34]
FTO/TiO2/N719/凝胶电解质/多壁碳纳米管/介孔活性炭/棉织物 刮涂法 12.3 0.72 0.685 6.06 [35]
FTO/TiO2/N719/凝胶电解质/多壁碳纳米管/介孔活性炭/涤纶织物 刮涂法 12.4 0.72 0.701 9 6.26 [35]
FTO/TiO2/N719/凝胶电解质/多壁碳纳米管/介孔活性炭/亚麻面料 刮涂法 12.7 0.73 0.626 2 5.80 [35]
FTO/TiO2/N719/I-- I 3 -/活性炭/石墨烯/莱赛尔织物/聚对苯二甲酸乙二醇酯 涂覆法 15.5 0.73 0.628 7.09 [36]
FTO/TiO2/N719/I-- I 3 -/聚吡咯/镀镍织物 涂覆法 7.85 0.74 0.66 3.83 [40]
FTO/TiO2/N719/I-- I 3 -/聚苯胺/碳纤维织物 涂覆法 12.1 0.675 0.47 3.81 [41]
硬质平面 FTO/ TiO2/Dye/I-- I 3 -/石墨烯/棉织物/FTO 涂覆法 14.75 0.66 0.709 2 6.93 [37]
FTO/ZnO/N719/I-- I 3 -/活性炭布/FTO 原子沉积 14.03 0.7499 0.655 6.88 [39]
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