Journal of Textile Research ›› 2022, Vol. 43 ›› Issue (02): 149-155.doi: 10.13475/j.fzxb.20211102207

• Dyeing and Finshing & Chemicals • Previous Articles     Next Articles

Low angle-dependent structurally coloured films over full visible spectrum

LIN Tiantian, YANG Dan, GAO Weihong(), ZHANG Zhiyue, ZHAO Xiaoyan   

  1. School of Textiles and Fashion, Shanghai University of Engineering Science, Shanghai 201620, China
  • Received:2021-11-03 Revised:2021-12-01 Online:2022-02-15 Published:2022-03-15
  • Contact: GAO Weihong E-mail:gaoweihong@sues.edu.cn

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Abstract:

In order to solve high pollution and energy consumption of traditional dyes, and prepare full visible spectral structural colours with no pollution, three batches of different sized (320, 240 and 200 nm) silica nanoparticles (SNPs) were synthesized by using a Stöber-based solvent varying method, the silica photonic crystal(PC) films were fabricated from the three sized bare SNPs with vivid red, green, and purple colours, respectively, and structurally coloured PC films over the full visible spectrum were fabricated by varying the mass ratio of two sized SNPs. The result showed that the structural colours of the PC films had a blue shift when the ratio of the smaller sized SNPs increased. The PC films consisting of non-uniform two sized SNPs showed low angle dependent structural colours, due to its amorphous PC structure. This method is simpler and faster than traditional self-assembly of PC materials that require a series of different sized microsphere bathes for each color, and is suitable for making stable colours as pigments and coatings on different substrates.

Key words: structural colour, photonic crystal, silica nanoparticle, full visible spectrum, low angle-dependence

CLC Number: 

  • TS190.2

Tab.1

Recipes for Sa, Sb and ScmL"

样品 EtOH NH3·H2O H2O TEOS
Sa 60 8 3 6
Sb 75 8 3 6
Sc 90 8 3 6

Fig.1

Fabrication procedure of full visible spectrum structurally coloured films"

Fig.2

Particle size distribution"

Fig.3

Spectral reflections(a) of films composed of Sa, Sb, Sc and photos(b) of PC films"

Fig.4

Optical photos (a) and spectral reflections (b) of PC films and relationship between Sb content and reflection peak wavelength(c)"

Fig.5

Average particle diameter(a) and CIE 1931 chromaticity diagram(b) of films"

Fig.6

SEM images and corresponding FFT images of PC films"

Fig.7

Spectral reflections of PC films observed at different viewing angles"

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